Long ranged stress correlations in the hard sphere liquid
Abstract
The smooth emergence of shear elasticity is an hallmark of the liquid to glass transition. In a liquid, viscous stresses arise from local structural rearrangements. In the solid, Eshelby has shown that stresses around an inclusion decay as a power law , where is the dimension of the system. We study glass-forming hard sphere fluids by simulation and observe the emergence of the unscreened power-law Eshelby pattern in the stress correlations of the isotropic liquid state. By a detailed tensorial analysis, we show that the fluctuating force field, viz.~the divergence of the stress field, relaxes to zero with time in all states, while the shear stress correlations develop spatial power-law structures inside regions that grow with longitudinal and transverse sound speeds; we observe the predicted exponents and . In Brownian systems, shear stresses relax diffusively within these regions, with the diffusion coefficient determined by the shear modulus and the friction coefficient.
Cite
@article{arxiv.2405.03497,
title = {Long ranged stress correlations in the hard sphere liquid},
author = {Niklas Grimm and Martin von Bischopinck and Andreas Zumbusch and Matthias Fuchs},
journal= {arXiv preprint arXiv:2405.03497},
year = {2024}
}
Comments
15 pages, 18 figures