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Long range order in the dipolar XY antiferromagnet Er$_2$Sn$_2$O$_7$

Strongly Correlated Electrons 2017-11-16 v2 Materials Science

Abstract

Er2_2Sn2_2O7_7 remains a puzzling case among the extensively studied frustrated compounds of the rare-earth pyrochlore family. Indeed, while a first order transition towards a long-range antiferromagnetic state with the so-called Palmer-Chalker structure is theoretically predicted, it has not been observed yet, leaving the issue, as to whether it is a spin-liquid candidate, open. We report on neutron scattering and magnetization measurements which evidence a second order transition towards this Palmer-Chalker ordered state around 108 mK. Extreme care was taken to ensure a proper thermalization of the sample, which has proved to be crucial to successfully observe the magnetic Bragg peaks. At the transition, a gap opens in the excitations, superimposed on a strong quasielastic signal. The exchange parameters, refined from a spin wave analysis in applied magnetic field, confirm that Er2_2Sn2_2O7_7 is a realization of the dipolar XY pyrochlore antiferromagnet. The proximity of competing phases and the strong XY anisotropy of the Er3+^{3+} magnetic moment might be at the origin of enhanced fluctuations, leading to the unexpected nature of the transition, the low ordering temperature, and the observed multi-scale dynamics.

Keywords

Cite

@article{arxiv.1705.04462,
  title  = {Long range order in the dipolar XY antiferromagnet Er$_2$Sn$_2$O$_7$},
  author = {S. Petit and E. Lhotel and F. Damay and P. Boutrouille and A. Forget and D. Colson},
  journal= {arXiv preprint arXiv:1705.04462},
  year   = {2017}
}

Comments

7 pages, 6 figures