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Local magnetic moments due to loop currents in metals

Strongly Correlated Electrons 2022-12-20 v2

Abstract

We present Hartree-Fock calculations on a simple model to obtain the conditions of formation of local magnetic moments due to loop-currents LoL_o and spin-loop currents LsL_s and compare them to the conditions of formation of local spin-moments MM which were given long ago in a similar approximation by Anderson. A model with three degenerate orbitals sitting on an equilateral triangle, with on-site and nearest-neighbor repulsions UU and VV respectively, and inter-site kinetic energy, hybridizing with conduction electrons with a parameter Δ{\Delta} is investigated. LoL_o and LsL_s are promoted by large V/ΔV/{\Delta} and their magnitude is relatively unaffected by U/ΔU/{\Delta}. Spin-magnetic moments MM promoted by large U/ΔU/{\Delta} on the other hand are adversely affected by V/ΔV/{\Delta}. In this model, LoL_o for VV multiplied by the number of neighbors is approximately the same as the MM promoted by UU in Anderson's local model for MM. LoL_o and LsL_s are degenerate if exchange interactions and Hund's rule are neglected but LoL_o is favored when they are included. Many of the qualitative results are visible in an expression for the Hartree-Fock ground state energy derived as a function of small Lo,LsL_o, L_s and MM. Numerical minimization of the Hartree-Fock energy is presented for larger values. We also briefly discuss the connection and differences of the interaction generated orbital currents and spin-currents discussed here and generalized to a lattice with the topological states in metals and semi-conductors.

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Cite

@article{arxiv.2208.05587,
  title  = {Local magnetic moments due to loop currents in metals},
  author = {Arkady Shekhter and Chandra M. Varma},
  journal= {arXiv preprint arXiv:2208.05587},
  year   = {2022}
}

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7 pages