English

Local geometry around B atoms in B/Si(111) from polarized x-ray absorption spectroscopy

Materials Science 2019-02-19 v1

Abstract

The arrangement of B~atoms in a doped Si(111)-(3×3)R30(\sqrt{3}\times\sqrt{3})R30^{\circ}:B system was studied using near-edge x-ray absorption fine structure (NEXAFS). Boron atoms were deposited via segregation from the bulk by flashing the sample repeatedly. The positions of B~atoms are determined by comparing measured polarized (angle-dependent) NEXAFS spectra with spectra calculated for various structural models based on ab-initio total energy calculations. It is found that most of boron atoms are located in sub-surface L1c_{1}^{c} positions, beneath a Si atom. However, depending on the preparation method a significant portion of B~atoms may be located elsewhere. A possible location of these non-L1c_{1}^{c}-atoms is at the surface, next to those Si atoms which form the (3×3)R30(\sqrt{3}\times\sqrt{3})R30^{\circ} reconstruction.

Keywords

Cite

@article{arxiv.1902.06244,
  title  = {Local geometry around B atoms in B/Si(111) from polarized x-ray absorption spectroscopy},
  author = {Saleem Ayaz Khan and Martin Vondráček and Peter Blaha and Kateřina Horáková and Jan Minár and Ondřej Šipr and Vladimír Cháb},
  journal= {arXiv preprint arXiv:1902.06244},
  year   = {2019}
}

Comments

9 pages, 8 figures