English

Local and collective magnetism of EuFe$_2$As$_2$

Superconductivity 2017-03-30 v1 Materials Science Strongly Correlated Electrons

Abstract

We present an experimental study of the local and collective magnetism of EuFe2As2\mathrm{EuFe_2As_2}, that is isostructural with the high temperature superconductor parent compound BaFe2As2\mathrm{BaFe_2As_2}. In contrast to BaFe2As2\mathrm{BaFe_2As_2}, where only Fe spins order, EuFe2As2\mathrm{EuFe_2As_2} has an additional magnetic transition below 20 K due to the ordering of the Eu2+^{2+} spins (J=7/2J =7/2, with L=0L=0 and S=7/2S=7/2) in an A-type antiferromagnetic texture (ferromagnetic layers stacked antiferromagnetically). This may potentially affect the FeAs layer and its local and correlated magnetism. Fe-Kβ_\beta x-ray emission experiments on EuFe2As2\mathrm{EuFe_2As_2} single crystals reveal a local magnetic moment of 1.3±0.15 μB\pm0.15~\mu_B at 15 K that slightly increases to 1.45±0.15 μB\pm0.15~\mu_B at 300 K. Resonant inelastic x-ray scattering (RIXS) experiments performed on the same crystals show dispersive broad (in energy) magnetic excitations along (0,0)(1,0)\mathrm{(0, 0)\rightarrow(1, 0)} and (0,0)(1,1)\mathrm{(0, 0)\rightarrow(1, 1)} with a bandwidth on the order of 170-180 meV. These results on local and collective magnetism are in line with other parent compounds of the AFe2As2\mathrm{AFe_2As_2} series (A=A= Ba, Ca, and Sr), especially the well characterized BaFe2As2\mathrm{BaFe_2As_2}. Thus, our experiments lead us to the conclusion that the effect of the high magnetic moment of Eu on the magnitude of both Fe local magnetic moment and spin excitations is small and confined to low energy excitations.

Keywords

Cite

@article{arxiv.1703.09819,
  title  = {Local and collective magnetism of EuFe$_2$As$_2$},
  author = {Pelliciari Jonathan and Ishii Kenji and Dantz Marcus and Lu Xingye and McNally Daniel and Strocov Vladimir and Xing Lingyi and Wang Xiancheng and Jin Changqing and Jeevan Hirale and Gegenwart Philipp and Schmitt Thorsten},
  journal= {arXiv preprint arXiv:1703.09819},
  year   = {2017}
}