Tailoring at will polar textures in ferroelectrics is critical for the development of nanoscale electronics and functional oxide technologies. Freestanding ferroelectric membranes have enabled studies of strain-induced polarization responses, but the control over membrane shape and local polarization typically remains limited to spontaneous buckling or uniaxial mechanical deformations. In this work, we employ a versatile photosensitive-polymer patterning approach to impose programmable bending strain profiles in ferroelectric membranes. Using BaTiO3 as a model system, we demonstrate deterministic 90{\deg} polarization rotation driven by engineered in-plane strain, and 180{\deg} polarization reversal arising from flexoelectric coupling through a controlled strain gradient. These results establish this programmable bending as a powerful approach to investigate strain-dependent domain structures, leverage flexoelectric effects, and engineer custom ferroelectric landscapes across a wide range of oxide membranes.
@article{arxiv.2511.19029,
title = {Light-induced photomechanical patterning of ferroelectric polarization},
author = {Alban Degezelle and Jonas Strobelt and Sarah Loebner and Moussa Mebarki and Stephane Fusil and Vincent Garcia and Bruno Berini and Vincent Polewczyk and Yves Dumont and Sylvia Matzen and Philippe Lecoeur and Svetlana Santer and Thomas Maroutian},
journal= {arXiv preprint arXiv:2511.19029},
year = {2025}
}
Comments
40 pages (double line spacing) and 13 figures, including the supporting information part