Lifetime of dynamical heterogeneity in a highly supercooled liquid
Abstract
We numerically examine dynamical heterogeneity in a highly supercooled three-dimensional liquid via molecular-dynamics simulations. To define the local dynamics, we consider two time intervals, and . is the relaxation time, and is the time at which non-Gaussian parameter of the van Hove self-correlation function is maximized. We determine the lifetimes of the heterogeneous dynamics in these two different time intervals, and , by calculating the time correlation function of the particle dynamics, i.e., the four-point correlation function. We find that the difference between and increases with decreasing temperature. At low temperatures, is considerably larger than , while remains comparable to . Thus, the lifetime of the heterogeneous dynamics depends strongly on the time interval.
Keywords
Cite
@article{arxiv.1006.3704,
title = {Lifetime of dynamical heterogeneity in a highly supercooled liquid},
author = {Hideyuki Mizuno and Ryoichi Yamamoto},
journal= {arXiv preprint arXiv:1006.3704},
year = {2012}
}
Comments
4pages, 6figures