English

Large decrease of fluctuations for supercooled water in hydrophobic nanoconfinement

Statistical Mechanics 2015-05-20 v2

Abstract

We study by Monte Carlo simulations a coarse-grained model of a water layer confined in a fixed disordered matrix of hydrophobic nanoparticles at different particle concentrations c. For c=0 (bulk water) we find a first order liquid-liquid phase transition (LLPT). For c>0 our simulations are consistent with a LLPT line ending in two critical points at low and high pressure P. For c=25% we find a dramatic decrease of compressibility K_T, thermal expansion coefficient \alpha_P, specific heat C_P at high P and low temperature T. Surprisingly, the effect is present also for c as low as 2.4%. We conclude that the higher the confinement, the lower the thermodynamic fluctuations and the more difficult it will be to detect the LLPT.

Keywords

Cite

@article{arxiv.1010.0693,
  title  = {Large decrease of fluctuations for supercooled water in hydrophobic nanoconfinement},
  author = {Elena G. Strekalova and Marco G. Mazza and H. Eugene Stanley and Giancarlo Franzese},
  journal= {arXiv preprint arXiv:1010.0693},
  year   = {2015}
}

Comments

11 pages with 4 figures

R2 v1 2026-06-21T16:23:37.357Z