English

Interaction-Driven Topological Transitions in Monolayer TaIrTe$_4$

Strongly Correlated Electrons 2025-06-25 v1 Mesoscale and Nanoscale Physics

Abstract

Discovering materials that combine topological phenomena with correlated electron behavior is a central pursuit in quantum materials research. Monolayer TaIrTe4_4 has recently emerged as a promising platform in this context, hosting robust quantum spin Hall insulator (QSHI) phases both within a single-particle gap and within a correlation-induced gap arising from van Hove singularities (vHSs), accessed via electrostatic doping. Its intrinsic monolayer nature offers exceptional tunability and the potential to realize a versatile array of interaction-driven topological phases. In this work, we combine theory and experiment to map the phase landscape of monolayer TaIrTe4_4. Using Hartree-Fock calculations, we investigate the interaction-driven phase diagram near the vHSs under commensurate filling conditions. By systematically tuning the dielectric screening and strain, we uncover a rich set of ground states--including QSHI, trivial insulator, higher-order topological insulator, and metallic phase--among which are interaction-driven topological phase transitions. Experimentally, we perform both local and nonlocal transport measurements across a broad set of devices, which--due to unavoidable strain variations during fabrication-realize several phases consistent with theoretical predictions. Together, our results lay the groundwork for understanding correlation-driven topological phenomena in TaIrTe4_4 and open new directions for engineering exotic quantum phases in low-dimensional materials beyond the limitations of moir\'e superlattices.

Keywords

Cite

@article{arxiv.2506.18412,
  title  = {Interaction-Driven Topological Transitions in Monolayer TaIrTe$_4$},
  author = {Jiangxu Li and Jian Tang and Louis Primeau and Thomas Siyuan Ding and Rahul Soni and Tiema Qian and Kenji Watanabe and Takashi Taniguchi and Ni Ni and Adrian Del Maestro and Qiong Ma and Yang Zhang},
  journal= {arXiv preprint arXiv:2506.18412},
  year   = {2025}
}

Comments

12+18 pages, 8+14 figures

R2 v1 2026-07-01T03:29:02.572Z