English

Integrating in-situ Shear Rheology with Neutron Reflectometry for Structural and Dynamic Analysis of Interfacial Systems

Applied Physics 2026-03-31 v2

Abstract

The study of the structure and mechanical properties of complex fluid interfaces has gained increasing interest in recent decades as a result of its significant scientific relevance to the understanding of biological systems, drug development, and industrial applications. The in situ combination of molecular-level structural measurements with the assessment of dynamical (rheological) properties is particularly valuable, as comparing measurements conducted on separate samples under challenging-to-reproduce experimental conditions can be problematic. In this work, we present a new sample environment at the FIGARO instrument, the horizontal neutron reflectometer at the Institut Laue-Langevin, which includes an interfacial shear rheometer operating in the Double Wall-Ring (DWR) geometry, compatible with commercial rotational rheometers. This innovative setup enables simultaneous structural (neutron reflectometry) and dynamical (shear interfacial rheology) measurements on the same sample.

Keywords

Cite

@article{arxiv.2411.04660,
  title  = {Integrating in-situ Shear Rheology with Neutron Reflectometry for Structural and Dynamic Analysis of Interfacial Systems},
  author = {P. Sanchez-Puga and J. Tajuelo and J. Carrascosa-Tejedor and M. A. Rubio and P. Gutfreund and A. Maestro},
  journal= {arXiv preprint arXiv:2411.04660},
  year   = {2026}
}

Comments

Author Accepted Manuscript of an article accepted for publication in Journal of Applied Crystallography, before journal formatting. Final version link will be added when available