Zintl phase EuIn2As2 has garnered growing attention as an axion insulator candidate, triggered by the identification of a commensurate double-Q broken-helix state in previous studies, however, its periodicity and symmetry remain subjects of debate. Here, we perform resonant x-ray scattering experiments on EuIn2As2, revealing an incommensurate nature of the broken-helix state, where both the wave number and the amplitude of the helical modulation exhibit systematic sample dependence. Furthermore, the application of an in-plane magnetic field brings about a fanlike state that appears to preserve the double-Q nature, which might be attributed to multiple-spin interactions in momentum space. We propose that the itinerant character of EuIn2As2, most likely induced by Eu deficiency, gives rise to the helical modulation and impedes the realization of a theoretically-predicted axion state with the collinear antiferromagnetic order.
@article{arxiv.2403.03022,
title = {Incommensurate broken helix induced by nonstoichiometry in the axion insulator candidate EuIn$_{2}$As$_{2}$},
author = {Masaki Gen and Yukako Fujishiro and Kazuki Okigami and Satoru Hayami and Max T. Birch and Kiyohiro Adachi and Daisuke Hashizume and Takashi Kurumaji and Hajime Sagayama and Hironori Nakao and Yoshinori Tokura and Taka-hisa Arima},
journal= {arXiv preprint arXiv:2403.03022},
year = {2025}
}
Comments
6 pages, 5 figures, SM: 13 pages, 9 figures, published in Phys. Rev. B