English

Impact of dipole-dipole interactions on motility-induced phase separation

Soft Condensed Matter 2022-03-29 v1 Statistical Mechanics

Abstract

We present a hydrodynamic theory for systems of dipolar active Brownian particles which, in the regime of weak dipolar coupling, predicts the onset of motility-induced phase separation (MIPS), consistent with Brownian dynamics (BD) simulations. The hydrodynamic equations are derived by explicitly coarse-graining the microscopic Langevin dynamics, thus allowing for a quantitative comparison of parameters entering the coarse-grained model and particle-resolved simulations. Performing BD simulations at fixed density, we find that dipolar interactions tend to hinder MIPS, as first reported in [Liao et al., Soft Matter, 2020, 16, 2208]. Here we demonstrate that the theoretical approach indeed captures the suppression of MIPS. Moreover, the analysis of the numerically obtained, angle-dependent correlation functions sheds light into the underlying microscopic mechanisms leading to the destabilization of the homogeneous phase.

Keywords

Cite

@article{arxiv.2203.13841,
  title  = {Impact of dipole-dipole interactions on motility-induced phase separation},
  author = {Elena Sesé-Sansa and Guo-Jun Liao and Demian Levis and Ignacio Pagonabarraga and Sabine H. L. Klapp},
  journal= {arXiv preprint arXiv:2203.13841},
  year   = {2022}
}

Comments

14 pages, 10 figures