English

High-resolution x-ray diffraction study of the heavy-fermion compound YbBiPt

Strongly Correlated Electrons 2015-12-07 v1

Abstract

YbBiPt is a heavy-fermion compound possessing significant short-range antiferromagnetic correlations below a temperature of T*=0.7T^{\textrm{*}}=0.7 K, fragile antiferromagnetic order below TN=0.4T_{\rm{N}}=0.4 K, a Kondo temperature of TK1T_{\textrm{K}} \approx1 K, and crystalline-electric-field splitting on the order of E/kB=1-10E/k_{\textrm{B}}=1\,\textrm{-}\,10 K. Whereas the compound has a face-centered-cubic lattice at ambient temperature, certain experimental data, particularly those from studies aimed at determining its crystalline-electric-field scheme, suggest that the lattice distorts at lower temperature. Here, we present results from high-resolution, high-energy x-ray diffraction experiments which show that, within our experimental resolution of 6-10×105\approx6\,\textrm{-}\,10\times10^{-5} \AA, no structural phase transition occurs between T=1.5T=1.5 and 5050 K. In combination with results from dilatometry measurements, we further show that the compound's thermal expansion has a minimum at 18\approx18 K and a region of negative thermal expansion for 9<T<189<T<18 K. Despite diffraction patterns taken at 1.61.6 K which indicate that the lattice is face-centered cubic and that the Yb resides on a crystallographic site with cubic point symmetry, we demonstrate that the linear thermal expansion may be modeled using crystalline-electric-field level schemes appropriate for Yb3+^{3+} residing on a site with either cubic or less than cubic point symmetry.

Keywords

Cite

@article{arxiv.1511.01822,
  title  = {High-resolution x-ray diffraction study of the heavy-fermion compound YbBiPt},
  author = {B. G. Ueland and S. M. Saunders and S. L. Bud'ko and G. M. Schmiedeshoff and P. C. Canfield and A. Kreyssig and A. I. Goldman},
  journal= {arXiv preprint arXiv:1511.01822},
  year   = {2015}
}

Comments

7 pages, 3 figures, submitted to Phys. Rev. B