English

Griffiths phase and critical behavior in layered Sr$_2$IrO$_4$ ferromagnet

Strongly Correlated Electrons 2016-08-10 v1 Materials Science Other Condensed Matter

Abstract

We report the existence of Griffiths phase (GP) and its influence on critical phenomena in layered Sr2_2IrO4_4 ferromagnet (TC_C = 221.5 K). The power law behavior of inverse magentic susceptibility, 1/χ\chi(T) with exponent λ=0.18(2)\lambda = 0.18(2) confirm the GP in the regime TC_C << T \leq TG_G = 279.0(5) K. Moreover, the detailed critical analysis via modified Arrott plot method exhibits unrealistic critical exponents β\beta = 0.77(1), γ\gamma = 1.59(2) and δ=3.06(4)\delta = 3.06(4), in corroboration with magneto-caloric study. The abnormal exponent values have been viewed in context of ferromagnetic-Griffiths phase transition. The GP has been further analyzed using Bray model, which yields a reliable value of β\beta = 0.19(2), belonging to the two-dimensional (2D) XYh4_4 universality class with strong anisotropy present in Sr2_2IrO4_4. The present study proposes Bray model as a possible tool to investigate the critical behavior for Griffiths ferromagnets in place of conventional Arrott plot analysis. The possible origins of GP and its correlation with insulating nature of Sr2_2IrO4_4 have been discussed.

Keywords

Cite

@article{arxiv.1608.02726,
  title  = {Griffiths phase and critical behavior in layered Sr$_2$IrO$_4$ ferromagnet},
  author = {A. Rathi and Sonam Perween and P. K. Rout and R. P. Singh and Anurag Gupta and Sukhvir Singh and B. Gahtori and B. Sivaiah and Ajay Dhar and A. K. Shukla and R. K. Rakshit and R. P. Pant and G. A. Basheed},
  journal= {arXiv preprint arXiv:1608.02726},
  year   = {2016}
}