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Giant Exfoliation Induced Magnetic Coercivity in Fe$_3$GaTe$_2$

Materials Science 2026-07-30 v1 Mesoscale and Nanoscale Physics

Abstract

Permanent magnets with strong anisotropy and high coercivity underpin modern information and energy technologies, yet rare-earth-free alternatives remain limited. Here, we show that thickness engineering via mechanical exfoliation induces hard magnetic behavior in the van der Waals ferromagnet Fe3_3GaTe2_2. Bulk crystals exhibit Curie temperatures above 350 K but negligible room-temperature coercivity. When thinned below 100 nm, the coercive field is dramatically enhanced, reaching nearly 1 T at room temperature for in-plane fields which is comparable to values of conventional hard magnets. Micromagnetic analysis reveals a crossover in magnetization reversal from domain-mediated processes in bulk samples to quasi-coherent rotation in thin flakes, driven by increased effective anisotropy and suppressed domain formation. This thickness-dependent transition enables tuning of magnetic hardness without chemical modification. Combined with high saturation magnetization and robust room-temperature performance, Fe3_3GaTe2_2 emerges as a promising rare-earth-free material for spintronic applications. Its layered structure further allows integration into van der Waals heterostructures, where large in-plane coercivity can stabilize magnetic states against perturbations and interlayer coupling, offering potential for high-density nonvolatile memory and domain-wall-based devices.

Keywords

Cite

@article{arxiv.2607.28828,
  title  = {Giant Exfoliation Induced Magnetic Coercivity in Fe$_3$GaTe$_2$},
  author = {Lingrui Mei and PeiYu Cai and Sang-Eon Lee and Yue Li and Shyam Raj Karullithodi and Vadym Kulichenko and Charudatta Pathak and Elton J. G. Santos and Luis Balicas},
  journal= {arXiv preprint arXiv:2607.28828},
  year   = {2026}
}

Comments

5 figures, plus Supplementary information, including 6 supplementary figures