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Gapped commensurate antiferromagnetic response in a strongly underdoped model cuprate superconductor

Superconductivity 2024-12-05 v1 Strongly Correlated Electrons

Abstract

It is a distinct possibility that spin fluctuations are the pairing interactions in a wide range of unconventional superconductors. In the case of the high-transition-temperature (high-TcT_c) cuprates, in which superconductivity emerges upon doping an antiferromagnetic Mott-insulating state, spin correlations might furthermore drive unusual pseudogap phenomena. Here we use polarized and unpolarized magnetic neutron scattering to study the simple tetragonal cuprate HgBa2CuO4+δ\mathrm{HgBa}_{2}\mathrm{CuO}_{4+\delta} at very low doping (Tc55T_c \approx 55 K, hole concentration p0.064p \approx 0.064). In stark contrast to prior results for other underdoped cuprates, we find no evidence of incommensurate spin-density-wave, charge-spin stripe, or q=0q = 0 magnetic order. Instead, the antiferromagnetic response in both the superconducting and pseudogap states is gapped below ΔAF6\Delta_\mathrm{AF} \approx 6 meV, commensurate over a wide energy range, and disperses above about 55 meV. Given the documented model nature of HgBa2CuO4+δ\mathrm{HgBa}_{2}\mathrm{CuO}_{4+\delta}, which exhibits high structural symmetry and minimal point disorder effects, we conclude that the observed behavior signifies the unmasked response of the quintessential CuO2\mathrm{CuO}_{2} planes near the Mott-insulating state. These results for HgBa2CuO4+δ\mathrm{HgBa}_{2}\mathrm{CuO}_{4+\delta} can therefore be expected to serve as a benchmark for a refined theoretical understanding of the cuprates.

Cite

@article{arxiv.2412.03524,
  title  = {Gapped commensurate antiferromagnetic response in a strongly underdoped model cuprate superconductor},
  author = {Zachary W. Anderson and Yang Tang and Vikram Nagarajan and Mun K. Chan and Chelsey J. Dorow and Guichuan Yu and Douglas L. Abernathy and Andrew D. Christianson and Lucile Mangin-Thro and Paul Steffens and Tyler Sterling and Dmitry Reznik and Dalila Bounoua and Yvan Sidis and Philippe Bourges and Martin Greven},
  journal= {arXiv preprint arXiv:2412.03524},
  year   = {2024}
}

Comments

Main text: 18 pages, 6 figures. Supplement: 17 pages, 10 figures