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Gapless dispersive continuum in a modulated quantum kagome antiferromagnet

Strongly Correlated Electrons 2024-11-26 v2 Materials Science Other Condensed Matter

Abstract

The pursuit of quantum spin liquid (QSL) states in condensed matter physics has drawn attention to kagome antiferromagnets (AFM) where a two-dimensional corner-sharing network of triangles frustrates conventional magnetic orders. While quantum kagome AFMs based on Cu2+^{2+} (3d9^9, s=12s=\frac{1}{2}) ions have been extensively studied, there is so far little work beyond copper-based systems. Here we present our bulk magnetization, specific heat and neutron scattering studies on single crystals of a new titanium fluoride Cs8_8RbK3_3Ti12_{12}F48_{48} where Ti3+^{3+} (3d1^1, s=12s = \frac{1}{2}) ions form a modulated quantum kagome antiferromagnet that does not order magnetically down to 1.5 K. Our comprehensive map of the dynamic response function S(Q,ω)S(Q,\hbar\omega) acquired at 1.5 K where the heat capacity is T-linear reveals a dispersive continuum emanating from soft lines that extend along (100). The data indicate fractionalized spinon-like excitations with quasi-one-dimensional dispersion within a quasi-two-dimensional spin system.

Keywords

Cite

@article{arxiv.2410.01931,
  title  = {Gapless dispersive continuum in a modulated quantum kagome antiferromagnet},
  author = {Asiri Thennakoon and Ryouga Yokokura and Yang Yang and Ryoichi Kajimoto and Mitsutaka Nakamura and Masahiro Hayashi and Chishiro Michioka and Gia-Wei Chern and Collin Broholm and Hiroaki Ueda and Seung-Hun Lee},
  journal= {arXiv preprint arXiv:2410.01931},
  year   = {2024}
}
R2 v1 2026-06-28T19:05:54.574Z