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Fractionalized Magnetization Plateaus in the Shastry-Sutherland Lattice Material Er$_2$Be$_2$GeO$_7$

Strongly Correlated Electrons 2024-12-06 v1

Abstract

The experimental study of magnetism on the Shastry-Sutherland lattice has been ongoing for more than two decades, following the discovery of the first Shastry-Sutherland lattice materials SrCu2_2(BO3_3)2_2. However, the study of Shastry-Sutherland systems is often complicated by the requirements of high magnetic fields (>>~20~T SrCu2_2(BO3_3)2_2) or the presence of itinerate electrons (e.g. REB4_4). In this paper, we present the magnetic properties of the Shastry-Sutherland lattice material Er2_2Be2_2GeO7_7. Like SrCu2_2(BO3_3)2_2, Er2_2Be2_2GeO7_7 exhibits fractionalized magnetization plateaus. Unlike SrCu2_2(BO3_3)2_2, Er2_2Be2_2GeO7_7 exhibits long-range order below 1 \sim1~K, and the plateaus are accessible using commercial laboratory equipment, occurring for fields <~1~T. The fractions of magnetization present are closest to 14\frac{1}{4} and 12\frac{1}{2} of the full powder moment; we show that the 14\frac{1}{4} magnetization plateau in Er2_2Be2_2GeO7_7 has a classical analog, well represented by the magnetic structure (canted antiferromagnetic) observed in powder neutron diffraction. The lack of itinerate electrons, chemical disorder, and the low fields required to access the fractionalized magnetization plateaus promises Er2_2Be2_2GeO7_7 to be a prime candidate for the study of frustrated magnetism on the Shastry-Sutherland lattice.

Keywords

Cite

@article{arxiv.2412.04360,
  title  = {Fractionalized Magnetization Plateaus in the Shastry-Sutherland Lattice Material Er$_2$Be$_2$GeO$_7$},
  author = {M. Pula and S. Sharma and J. Gautreau and Sajilesh K. P. and A. Kanigel and C. R. dela Cruz and T. N. Dolling and L. Clark and G. M. Luke},
  journal= {arXiv preprint arXiv:2412.04360},
  year   = {2024}
}

Comments

9 pages, 8 figures