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Fractionalization on the Surface: Is Type-II Terminated $1T$-TaS$_2$ Surface an Anomalously Realized Spin Liquid?

Strongly Correlated Electrons 2022-07-04 v3 Mesoscale and Nanoscale Physics Materials Science Superconductivity

Abstract

The type-II terminated 1T1T-TaS2_2 surface of a three-dimensional 1T1T-TaS2_2 bulk material realizes the effective spin-1/21/2 degree of freedom on each David star cluster with T2=1{\mathcal{T}^2=-1} such that the time-reversal symmetry is realized anomalously, despite the fact that bulk three-dimensional 1T1T-TaS2_2 material has an even number of electrons per unit cell with T2=+1{\mathcal{T}^2=+1}. This surface is effectively viewed as a spin-1/21/2 triangular lattice magnet, except with a fully gapped topological bulk. We further propose this surface termination realizes a spinon Fermi surface spin liquid with the surface fractionalization but with a nonexotic three-dimensional bulk. We analyze possible experimental consequences, especially the surface spectroscopic measurements, of the type-II terminated surface spin liquid.

Keywords

Cite

@article{arxiv.2109.08093,
  title  = {Fractionalization on the Surface: Is Type-II Terminated $1T$-TaS$_2$ Surface an Anomalously Realized Spin Liquid?},
  author = {Chao-Kai Li and Xu-Ping Yao and Jianpeng Liu and Gang Chen},
  journal= {arXiv preprint arXiv:2109.08093},
  year   = {2022}
}

Comments

Main text: 7 pages + 4 figures; Supplemental Material: 14 pages + 7 figures, including calculation details and more discussions