English

Finite-size effects in the nonphononic density of states in computer glasses

Soft Condensed Matter 2020-03-25 v2

Abstract

The universal form of the density of nonphononic, quasilocalized vibrational modes of frequency ω\omega in structural glasses, D(ω){\cal D}(\omega), was predicted theoretically decades ago, but only recently revealed in numerical simulations. In particular, it has been recently established that, in generic computer glasses, D(ω){\cal D}(\omega) increases from zero frequency as ω4\omega^4, independent of spatial dimension and of microscopic details. However, in [E. Lerner, and E. Bouchbinder, Phys. Rev. E 96, 020104(R) (2017)] it was shown that the preparation protocol employed to create glassy samples may affect the form of their resulting D(ω){\cal D}(\omega): glassy samples rapidly quenched from high temperature liquid states were shown to feature D(ω) ⁣ ⁣ωβ{\cal D}(\omega)\!\sim\!\omega^\beta with β ⁣< ⁣4\beta\!<\!4, presumably limiting the degree of universality of the ω4\omega^4 law. Here we show that exponents β ⁣< ⁣4\beta\!<\!4 are only seen in small glassy samples quenched from high-temperatue liquid states --- whose sizes are comparable to or smaller than the size of the disordered core of soft quasilocalized vibrations --- while larger glassy samples made with the same protocol feature the universal ω4\omega^4 law. Our results demonstrate that observations of β ⁣< ⁣4\beta\!<\!4 in the nonphononic density of states stem from finite-size effects, and we thus conclude that the ω4\omega^4 law should be featured by any sufficiently large glass quenched from a melt.

Keywords

Cite

@article{arxiv.1911.12741,
  title  = {Finite-size effects in the nonphononic density of states in computer glasses},
  author = {Edan Lerner},
  journal= {arXiv preprint arXiv:1911.12741},
  year   = {2020}
}

Comments

5 pages, 3 figures. v2: data for larger systems included in fig.3