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Ferroelectric switchable altermagnetic-like compensated ferrimagnets with charge ordering

Materials Science 2026-07-29 v1 Mesoscale and Nanoscale Physics Strongly Correlated Electrons

Abstract

Unconventional collinear magnets with almost zero magnetization but prominent nonrelativistic spin-splitting, such as altermagnets, can inherit the advantages of both ferromagnets and antiferromagnets. By incorporating more degrees of freedom such as ferroelectricity and charge ordering, these unconventional magnets can be even more interesting and functionalized. With this design principle, the Fe3_3O5_5 monolayer is predicted to exhibit a hybrid spin-splitting mechanism, with the superposition of the altermagnetic-like kk-path alternating splitting and ferrimagnet-like Zeeman splitting. Benefiting from the hidden magnetoelectricity based on the spin-charge coupling, such spin-splitting can be fully switched by an electric field. Its conductivity is highly spin-polarized, with a polarization ratio above 99%99\%, comparable to half-metals but with zero magnetization.

Cite

@article{arxiv.2607.26971,
  title  = {Ferroelectric switchable altermagnetic-like compensated ferrimagnets with charge ordering},
  author = {Xinyu Yang and Shuai Dong},
  journal= {arXiv preprint arXiv:2607.26971},
  year   = {2026}
}

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