English

Fermi surface and effective masses of IrO$_2$ probed by de Haas-van Alphen quantum oscillations

Strongly Correlated Electrons 2025-06-12 v1 Materials Science

Abstract

Iridium-containing conducting materials are widely investigated for their strong spin-orbit coupling and potential topological properties. Recently the commonly used electrode material iridium dioxide was found to host a large spin-Hall conductivity and was shown to support Dirac nodal lines. Here we present quantum-oscillation experiments on high-quality IrO2_2 single crystals using the de Haas-van Alphen effect measured using torque magnetometry with a piezo-resistive microcantilever as well as density functional theory-based band-structure calculations. The angle, temperature and field dependencies of the oscillations and the calculated band dispersion provide valuable information on the properties of the charge carriers, including the Fermi-surface geometry and electronic correlations. Comparison of experimental results to calculations allows us to assigns the observed de Haas-van Alphen frequencies to the calculated Fermi surface topology. We find that the effective masses of IrO2_2 are enhanced compared to the rest electron mass mem_e, ranging from 1.9 to 3.0~mem_e, whereas the scattering times indicate excellent sample quality. We discuss our results in context with recent ARPES and band-structure calculation results that found Dirac nodal lines in IrO2_2 and compare the effective masses and other electronic properties to those of similar materials like the nodal chain metal ReO2_2 in which Dirac electrons with very light effective masses have been observed.

Keywords

Cite

@article{arxiv.2506.09815,
  title  = {Fermi surface and effective masses of IrO$_2$ probed by de Haas-van Alphen quantum oscillations},
  author = {Kathrin Götze and Matthew J. Pearce and Suchit Negi and Jian-Rui Soh and Dharmalingam Prabhakaran and Paul A. Goddard},
  journal= {arXiv preprint arXiv:2506.09815},
  year   = {2025}
}

Comments

7 pages, 5 figures