English

Fermi liquid state and enhanced electron correlations in the new iron pnictide CaFe$_4$As$_3$

Strongly Correlated Electrons 2009-04-28 v1

Abstract

The newly discovered CaFe4_4As3_3 system displays low-temperature Fermi liquid behavior, with enhanced electron-electron correlations. At high temperatures, the magnetic susceptibility shows Curie-Weiss behavior, with a large temperature-independent contribution. Antiferromagnetic ordering is observed below TN_N = (88.0 ±\pm 1.0) K, possibly via a spin density wave (SDW) transition. A remarkably sharp drop in resistivity occurs below T2_2 = (26.4 ±\pm 1.0) K, correlated with a similarly abrupt increase in the susceptibility, but no visible feature in the specific heat. The electronic specific heat coefficient γ\gamma at low temperatures is close to 0.02 J molFe1^{-1}_{Fe} K2^{-2}, but a higher value for γ\gamma (\sim0.08 J molFe1^{-1}_{Fe} K2^{-2} can be inferred from a linear C/ / T \textit{vs.} T2^2 just above T2_2. The Kadowaki-Woods ratio A/γ2/\gamma^2 = 55105*10^{-5} μΩ\mu \Omegacm mol2^2 K2^2 mJ2^{-2} is nearly two orders of magnitude larger than that of heavy fermions.

Keywords

Cite

@article{arxiv.0904.4188,
  title  = {Fermi liquid state and enhanced electron correlations in the new iron pnictide CaFe$_4$As$_3$},
  author = {Liang L. Zhao and Tanghong Yi and James C. Fettinger and Susan M. Kauzlarich and E. Morosan},
  journal= {arXiv preprint arXiv:0904.4188},
  year   = {2009}
}