Experimental high-dimensional entanglement certification and quantum steering with time-energy measurements

High-dimensional entanglement provides unique ways of transcending the limitations of current approaches in quantum information processing, quantum communications based on qubits. The generation of time-frequency qudit states offer significantly increased quantum capacities while keeping the number of photons constant, but pose significant challenges regarding the possible measurements for certification of entanglement. Here, we develop a new scheme and experimentally demonstrate the certification of 24-dimensional entanglement and a 9-dimensional quantum steering. We then subject our photon-pairs to dispersion conditions equivalent to the transmission through 600-km of fiber and still certify 21-dimensional entanglement. Furthermore, we use a steering inequality to prove 7-dimensional entanglement in a semi-device independent manner, proving that large chromatic dispersion is not an obstacle in distributing and certifying high-dimensional entanglement and quantum steering. Our approach, leveraging intrinsic large-alphabet nature of telecom-band photons, enables scalable, commercially viable, and field-deployable entangled and steerable quantum sources, providing a pathway towards fully scalable quantum information processer and high-dimensional quantum communication networks.