English

Exchange energy of the ferromagnetic electronic ground-state in a monolayer semiconductor

Strongly Correlated Electrons 2023-11-07 v1 Mesoscale and Nanoscale Physics

Abstract

Mobile electrons in the semiconductor monolayer-MoS2_2 form a ferromagnetic state at low temperature. The Fermi sea consists of two circles, one at the KK-point, the other at the K~\tilde{K}-point, both with the same spin. Here, we present an optical experiment on gated MoS2_2 at low electron-density in which excitons are injected with known spin and valley quantum numbers. The resulting trions are identified using a model which accounts for the injection process, the formation of antisymmetrized trion states, electron-hole scattering from one valley to the other, and recombination. The results are consistent with a complete spin polarization. From the splittings between different trion states, we measure the exchange energy, Σ\Sigma, the energy required to flip a single spin within the ferromagnetic state, as well as the intervalley Coulomb exchange energy, JJ. We determine Σ=11.2\Sigma=11.2\,meV and J=5J=5\,meV at n=1.5×1012n=1.5 \times 10^{12}\,cm2^{-2}, and find that JJ depends strongly on the electron density, nn.

Keywords

Cite

@article{arxiv.2311.02164,
  title  = {Exchange energy of the ferromagnetic electronic ground-state in a monolayer semiconductor},
  author = {Nadine Leisgang and Dmitry Miserev and Hinrich Mattiat and Lukas Schneider and Lukas Sponfeldner and Kenji Watanabe and Takashi Taniguchi and Martino Poggio and Richard J. Warburton},
  journal= {arXiv preprint arXiv:2311.02164},
  year   = {2023}
}

Comments

13 pages, 11 figures