English

Exact closure and solution for spatial correlations in single-file diffusion

Statistical Mechanics 2022-02-02 v2

Abstract

Single-file transport, where particles diffuse in narrow channels while not overtaking each other, is a fundamental model for the tracer subdiffusion observed in confined systems, such as zeolites or carbon nanotubes. This anomalous behavior originates from strong bath-tracer correlations in 1D, which, despite extensive effort, have however remained elusive, because they involve an infinite hierarchy of equations. Here, for the Symmetric Exclusion Process, a paradigmatic model of single-file diffusion, we break the hierarchy and unveil a closed exact equation satisfied by these correlations, which we solve. Beyond quantifying the correlations, the central role of this key equation as a novel tool for interacting particle systems is further demonstrated by showing that it applies to out-of equilibrium situations, other observables and other representative single-file systems.

Keywords

Cite

@article{arxiv.2110.09269,
  title  = {Exact closure and solution for spatial correlations in single-file diffusion},
  author = {Aurélien Grabsch and Alexis Poncet and Pierre Rizkallah and Pierre Illien and Olivier Bénichou},
  journal= {arXiv preprint arXiv:2110.09269},
  year   = {2022}
}

Comments

Updated version. To appear in Science Advances

R2 v1 2026-06-24T06:58:29.766Z