English

Evolution of electronic structure in pristine and hole-doped kagome metal RbV$_3$Sb$_5$

Superconductivity 2022-02-23 v1

Abstract

We report on in situ low-temperature (4 K) scanning tunneling microscope measurements of atomic and electronic structures of the cleaved surfaces of an alkali-based kagome metal RbV3_3Sb5_5 single crystals. We find that the dominant pristine surface exhibits Rb-1x1 structure, in which a unique unidirectional 3a0\sqrt{3}a_0 charge order is discovered. As the sample temperature slightly rises, Rb-3\sqrt{3}x1 and Rb-3\sqrt{3}x3\sqrt{3} reconstructions form due to desorption of surface Rb atoms. Our conductance mapping results demonstrate that Rb desorption not only gives rise to hole doping, but also renormalizes the electronic band structures. Surprisingly, we find a ubiquitous gap opening near the Fermi level in tunneling spectra on all the surfaces despite their large differences of hole-carrier concentration, indicating an orbital-selective band reconstruction in RbV3_3Sb5_5.

Keywords

Cite

@article{arxiv.2109.11286,
  title  = {Evolution of electronic structure in pristine and hole-doped kagome metal RbV$_3$Sb$_5$},
  author = {Jiawei Yu and Kebin Xiao and Yonghao Yuan and Qiangwei Yin and Zhiqiang Hu and Chunsheng Gong and Yunkai Guo and Zhijun Tu and Hechang Lei and Qi-Kun Xue and Wei Li},
  journal= {arXiv preprint arXiv:2109.11286},
  year   = {2022}
}

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