English

Electronic correlation assisted ferroelectric metallic state in LiOsO$_3$

Strongly Correlated Electrons 2016-05-04 v1

Abstract

LiOsO3_3 has been recently identified as the first unambiguous "ferroelectric metal", experimentally realizing a prediction from 1965 by Anderson and Blount. In this work, we investigate the metallic state in LiOsO3_3 by means of infrared spectroscopy supplemented by Density Functional Theory and Dynamical Mean Field Theory calculations. Our measurements and theoretical calculations clearly show that LiOsO3_3 is a very bad metal with a small quasiparticle weight, close to a Mott-Hubbard localization transition. The agreement between experiments and theory allows us to ascribe all the relevant features in the optical conductivity to strong electron-electron correlations within the t2gt_{2g} manifold of the osmium atoms.

Keywords

Cite

@article{arxiv.1509.01785,
  title  = {Electronic correlation assisted ferroelectric metallic state in LiOsO$_3$},
  author = {I. Lo Vecchio and G. Giovannetti and M. Autore and P. Di Pietro and A. Perucchi and J. He and K. Yamaura and M. Capone and S. Lupi},
  journal= {arXiv preprint arXiv:1509.01785},
  year   = {2016}
}

Comments

5 pages, 3 figures

R2 v1 2026-06-22T10:50:06.487Z