Electric-field-driven resistive transition in multiferroic SrCo$_2$Fe$_{16}$O$_{27}$/Sr$_3$Co$_2$Fe$_{24}$O$_{41}$composite
Abstract
We report observation of electric-field-driven resistive transition at a characteristic threshold field across a temperature range 10-200 K in an off-stoichiometric composite of (~80 vol%) W- and (~20 vol%) Z-type hexaferrites. The dielectric constant and the relaxation time constant too exhibit anomalous jump at . The , the extent of jump in resistivity (), and the hysteresis associated with the jump [] are found to decrease systematically with the increase in temperature (). Several temperature-driven phase transitions have also been noticed in low and high resistive states (LRS and HRS). The temperature-driven conduction turns out to be governed by activated hopping of small polarons at all the phases with electric () and magnetic () field dependent activation energy . Interestingly, as the temperature is raised, the -driven conduction at a fixed temperature evolves from to across 10-200 K and within 110-200 K, follows three-dimensional variable range hopping (3D-VRH) with stretched exponential or power law ( varies within 0.6-0.7 and 0.6-0.8 at LRS and HRS, respectively) dependence depending on the localization length () to diffusion length () ratio associated with -driven conduction. The follows universal scaling only at LRS within 10-110 K but not at higher temperature or at HRS. The entire set of observations has been discussed within the framework of structural evolution of the point-defect (cation vacancies or oxygen excess) network. This comprehensive map of esoteric and patterns provides insights on defect driven effects in a composite useful for tuning both the resistive transition and multiferroicity.
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Cite
@article{arxiv.2112.06246,
title = {Electric-field-driven resistive transition in multiferroic SrCo$_2$Fe$_{16}$O$_{27}$/Sr$_3$Co$_2$Fe$_{24}$O$_{41}$composite},
author = {Shubhankar Mishra and Chandan K. Ghosh and Aditi Sahoo and Dipten Bhattacharya and Suchandal Mondal and P. Mandal},
journal= {arXiv preprint arXiv:2112.06246},
year = {2022}
}
Comments
12 pages, 9 figures