English

Electric field controlled spin transport in a topological insulator interfaced with a ferroelectric antiferromagnet

Mesoscale and Nanoscale Physics 2026-07-15 v1 Materials Science

Abstract

Topological insulators have been explored extensively for spin-charge interconversion via magnetic interfaces, yet the true response of their spin-charge conversion, particularly in the absence of an external magnetic field, remains to be studied. Here, we report electric-field control of spin-charge conversion in the topological insulator Bi2_2Te3_3 with the antiferromagnetic multiferroic BiFeO3_3, employing a nonlocal spin transport device. A systematic thickness dependence of the spin transport across the interface between Bi2_2Te3_3 and BiFeO3_3 reveals a signature of topological surface-state-dominated spin transport in the bilayer system. The spin-charge conversion remains robust for thicknesses above 10 nm but falls rapidly with reducing thickness and vanishes at 5 nm. This is consistent with the hybridization-induced emergence of a trivial insulating phase, which is supported by the coherency factor estimated from the magnetoconductance of Bi2_2Te3_3. These results establish that spin-momentum-locked surface states dominate interfacial spin transport in the decoupled regime. Beyond presenting efficient spin-charge interconversion at an entirely insulating magnetic interface, this work also highlights sputter-deposited Bi2_2Te3_3 as a high-quality and scalable platform for integrating quantum materials into devices. The nonlocal spin transport approach presented here provides a simple and direct evidence of spin-charge conversion and opens an efficient and practical pathway toward designing energy-efficient spin-based devices.

Keywords

Cite

@article{arxiv.2607.14031,
  title  = {Electric field controlled spin transport in a topological insulator interfaced with a ferroelectric antiferromagnet},
  author = {Yogesh Kumar and Pushpendra Gupta and Xinyan Li and Richa Mudgal and Ashish Omar and Ryan Chen and Mito Funatsu and Maya Ramesh and Nicholas Reiterer and Yuanqi Lyu and Yiping Zeng and Darrell G. Schlom and Alessandra Lanzara and Robert J. Birgeneau and James G. Analytis and Ramamoorthy Ramesh and Sajid Husain},
  journal= {arXiv preprint arXiv:2607.14031},
  year   = {2026}
}

Comments

23 pages, 4 Figures