English

Effect of A-site ionic radius on metamagnetic transition in charge ordered $Sm_{0.5}(Ca_{0.5-y}Sr_{y})MnO_3$ compounds

Materials Science 2019-03-28 v1 Strongly Correlated Electrons

Abstract

We investigate the ultra-sharp jump in the isothermal magnetization and the resistivity in the polycrystalline Sm0.5(Ca0.5ySry)MnO3Sm_{0.5}(Ca_{0.5-y}Sr_{y})MnO_3 (y=0,0.1,0.2,0.25,0.3,0.5)(y = 0, 0.1, 0.2, 0.25, 0.3, 0.5) compounds. The critical field (Hcr)(H_{cr}), required for the ultra-sharp jump, decreases with increase of `Sr' concentration, i.e. with increase of average A-site ionic radius rA\langle r_A\rangle. The magnetotransport data indicate that the phase separation increases with the increase of rA\langle r_A\rangle, i.e. with yy. The dependency of HcrH_{cr} with magnetic field sweep rate reveals that the ultra-sharp jump from antiferromagnetic (AFM) state to the ferromagnetic (FM) state is of martensitic in nature. Our two-band double exchange model Hamiltonian calculations show that the `Sr' doping induces the ferromagnetic clusters in the antiferromagnetic insulating phase and in turn reduces the critical field. In the end we present a phenomenological picture obtained from our combined experimental and theoretical study.

Keywords

Cite

@article{arxiv.1903.11348,
  title  = {Effect of A-site ionic radius on metamagnetic transition in charge ordered $Sm_{0.5}(Ca_{0.5-y}Sr_{y})MnO_3$ compounds},
  author = {Sanjib Banik and Kalpataru Pradhan and I. Das},
  journal= {arXiv preprint arXiv:1903.11348},
  year   = {2019}
}