We investigate the effect of Dzyaloshinskii-Moriya interactions on the low temperature magnetic susceptibility for a system whose low energy physics is dominated by short-range valence bonds (singlets). Our general perturbative approach is applied to specific models expected to be in this class, including the Shastry-Sutherland model of the spin-dimer compound SrCu_2(BO_3)_2 and the antiferromagnetic Heisenberg model of the recently discovered S=1/2 kagome compound ZnCu_3(OH)_6Cl_2. The central result is that a short-ranged valence bond phase, when perturbed with Dzyaloshinskii-Moriya interactions, will remain time-reversal symmetric in the absence of a magnetic field but the susceptibility will be nonzero in the T\to 0 limit. Applied to ZnCu_3(OH)_6Cl_2, this model provides an avenue for reconciling experimental results, such as the lack of magnetic order and lack of any sign of a spin gap, with known theoretical facts about the kagome Heisenberg antiferromagnet.
@article{arxiv.0809.0031,
title = {Dzyaloshinskii-Moriya interactions in valence bond systems},
author = {Mayra Tovar and Kumar S. Raman and Kirill Shtengel},
journal= {arXiv preprint arXiv:0809.0031},
year = {2009}
}
Comments
15 pages, 7 figures; An error in version 2 has been corrected which changes our conclusions (Eq. 8 of version 2 does not apply for systems that do not conserve spin)