English

Dynamics of active liquid interfaces

Soft Condensed Matter 2022-08-15 v1 Materials Science Chaotic Dynamics Fluid Dynamics

Abstract

Controlling interfaces of phase separating fluid mixtures is key to creating diverse functional soft materials. Traditionally, this is accomplished with surface-modifying chemical agents. Using experiment and theory, we study how mechanical activity shapes soft interfaces that separate an active and a passive fluid. Chaotic flows in the active fluid give rise to giant interfacial fluctuations and non-inertial propagating active waves. At high activities, stresses disrupt interface continuity and drive droplet generation, producing an emulsion-like active state comprised of finite-sized droplets. When in contact with a solid boundary, active interfaces exhibit non-equilibrium wetting transitions, wherein the fluid climbs the wall against gravity. These results demonstrate the promise of mechanically driven interfaces for creating a new class of soft active matter.

Keywords

Cite

@article{arxiv.2208.06044,
  title  = {Dynamics of active liquid interfaces},
  author = {Raymond Adkins and Itamar Kolvin and Zhihong You and Sven Witthaus and M. Cristina Marchetti and Zvonimir Dogic},
  journal= {arXiv preprint arXiv:2208.06044},
  year   = {2022}
}

Comments

62 pages, 5 figures, 13 supplementary figures

R2 v1 2026-06-25T01:39:23.362Z