We investigate the electronic structure of (Sr1−xLax)2RhO4 using a combination of the density functional and dynamical mean-field theories. Unlike the earlier local density approximation plus Hubbard U (LDA+U) studies, we find no sizable enhancement of the spin-orbit splitting due to electronic correlations and show that such an enhancement is a spurious effect of the static mean-field approximation of the LDA+U method. The electron doping suppresses the importance of electronic correlations, which is reflected in quasi-particle bandwidth increasing with x. (Sr1−xLax)2RhO4 can be classified as weakly correlated metal, which becomes an itinerant in-plane ferromagnet (but possibly A-type antiferromagnet) due to Stoner instability around x=0.2.
@article{arxiv.1412.4766,
title = {Doping-dependent bandwidth renormalization and spin-orbit coupling in (Sr$_{1-x}$La$_x$)$_2$RhO$_4$},
author = {Kyo-Hoon Ahn and Kwan-Woo Lee and Jan Kunes},
journal= {arXiv preprint arXiv:1412.4766},
year = {2015}
}
Comments
Corrected a factor of 2 error in our definition of doping x