English

Does frequency-temperature superposition hold in deeply super-cooled liquids?

Disordered Systems and Neural Networks 2007-05-23 v1 Soft Condensed Matter

Abstract

The temperature evolution of the broadband 10610^{-6}-101010^{10} Hz dielectric susceptibility of the paradigmatic glass formers glycerol, propylene carbonate, and fluoro-aniline is analyzed assuming a three-step relaxation due to the α\alpha-process, its excess wing, and a β\beta-process. We find that the α\alpha-peak and the wing can be described by susceptibility functions with temperature-independent high-frequency exponents, while the relative weight of these contributions does depend on the temperature. The excess wing and the β\beta-process are distinct phenomena; in particular, the relaxation strength of the excess wing grows with decreasing the temperature, contrary to that of the β\beta-process. In our interpretation, the frequency-temperature superposition of the α\alpha-process is valid for all temperatures; in the case of glycerol, a typical β\beta-process is unambiguously identified for the first time.

Keywords

Cite

@article{arxiv.cond-mat/0604597,
  title  = {Does frequency-temperature superposition hold in deeply super-cooled liquids?},
  author = {Catalin Gainaru and Alexander Brodin and Vladimir Novikov and Ernst A. Rössler},
  journal= {arXiv preprint arXiv:cond-mat/0604597},
  year   = {2007}
}

Comments

5 pages, 4 figures