English

Diluted paramagnetic impurities in nonmagnetic Ba$_2$YIrO$_6$

Strongly Correlated Electrons 2017-10-10 v3

Abstract

The cubic double perovskite Ba2_2YIrO6_6 has been investigated by the local probe techniques nuclear magnetic resonance (89^{89}Y NMR) and muon spin rotation (muSR). Both methods confirm the absence of magnetic long-range order in this compound but find evidence for diluted localized paramagnetic moments. NMR spin-lattice relaxation rate 1/T1 measurements suggest a slowing down of localized spin moments at low temperatures. An increase of the muSR spin-lattice relaxation rate lambda confirms the presence of weak magnetism in Ba2_2YIrO6_6 . However, these findings cannot be explained by the recently suggested excitonic type of magnetism. Instead, they point towards tiny amounts of localized paramagnetic spin centers leading to this magnetic response on the background of a simple nonmagnetic ground state of the 5d4^4 (J=0)J=0) electronic configuration of Ir5+^{5+}.

Keywords

Cite

@article{arxiv.1707.06027,
  title  = {Diluted paramagnetic impurities in nonmagnetic Ba$_2$YIrO$_6$},
  author = {F. Hammerath and R. Sarkar and S. Kamusella and C. Baines and H. -H. Klauss and T. Dey and A. Maljuk and S. Gaß and A. U. B. Wolter and H. -J. Grafe and S. Wurmehl and B. Büchner},
  journal= {arXiv preprint arXiv:1707.06027},
  year   = {2017}
}

Comments

8 pages, 7 figures