We demonstrate that combining standing-wave (SW) excitation with resonant inelastic x-ray scattering (RIXS) can lead to depth resolution and interface sensitivity for studying orbital and magnetic excitations in correlated oxide heterostructures. SW-RIXS has been applied to multilayer heterostructures consisting of a superconductor La1.85Sr0.15CuO4(LSCO) and a half-metallic ferromagnet La0.67Sr0.33MnO3 (LSMO). Easily observable SW effects on the RIXS excitations were found in these LSCO/LSMO multilayers. In addition, we observe different depth distribution of the RIXS excitations. The magnetic excitations are found to arise from the LSCO/LSMO interfaces, and there is also a suggestion that one of the dd excitations comes from the interfaces. SW-RIXS measurements of correlated-oxide and other multilayer heterostructures should provide unique layer-resolved insights concerning their orbital and magnetic excitations, as well as a challenge for RIXS theory to specifically deal with interface effects.
@article{arxiv.1802.09743,
title = {Depth-resolved resonant inelastic x-ray scattering at a superconductor/half-metallic ferromagnet interface through standing-wave excitation},
author = {Cheng-Tai Kuo and Shih-Chieh Lin and Giacomo Ghiringhelli and Yingying Peng and Gabriella Maria De Luca and Daniele Di Castro and Davide Betto and Mathias Gehlmann and Tom Wijnands and Mark Huijben and Julia Meyer-Ilse and Eric Gullikson and Jeffrey B. Kortright and Arturas Vailionis and Nicolas Gauquelin and Johan Verbeeck and Timm Gerber and Giuseppe Balestrino and Nicholas B. Brookes and Lucio Braicovich and Charles S. Fadley},
journal= {arXiv preprint arXiv:1802.09743},
year = {2018}
}
Comments
18 pages, 3 figures, plus supplemental materials (14 pages)