Depletion of two-level systems in ultrastable computer-generated glasses
Abstract
Amorphous solids exhibit quasi-universal low-temperature anomalies whose origin has been ascribed to localized tunneling defects. Using an advanced Monte Carlo procedure, we create {\it in silico} glasses spanning from hyperquenched to ultrastable glasses. Using a multidimensional path-finding protocol, we locate tunneling defects with energy splittings smaller than , with the temperature below which quantum effects are relevant (K in most experiments). We find that as the stability of a glass increases, its energy landscape as well as the manner in which it is probed tend to deplete the density of tunneling defects, as observed in recent experiments. We explore the real-space nature of tunneling defects, and find that they are mostly localized to a few atoms, but are occasionally dramatically delocalized.
Keywords
Cite
@article{arxiv.1910.11168,
title = {Depletion of two-level systems in ultrastable computer-generated glasses},
author = {Dmytro Khomenko and Camille Scalliet and Ludovic Berthier and David R. Reichman and Francesco Zamponi},
journal= {arXiv preprint arXiv:1910.11168},
year = {2020}
}
Comments
6 pages, 4 figures + Supplementary Material