English

Depinning dynamics of confined colloidal dispersions under oscillatory shear

Soft Condensed Matter 2023-01-25 v3

Abstract

Strongly confined colloidal dispersions under shear can exhibit a variety of dynamical phenomena, including depinning transitions and complex structural changes. Here, we investigate the behaviour of such systems under pure oscillatory shearing with shear rate γ˙(t)=γ˙0cos(ωt)\dot{\gamma}(t) = \dot{\gamma}_0 \cos(\omega t), as it is a common scenario in rheological experiments. The colloids' depinning behaviour is assessed from a particle level based on trajectories, obtained from overdamped Brownian Dynamics simulations. The numerical approach is complemented by an analytic one based on an effective single-particle model in the limits of weak and strong driving. Investigating a broad spectrum of shear rate amplitudes γ˙0\dot{\gamma}_0 and frequencies ω\omega, we observe complete pinning as well as temporary depinning behaviour. We discover that temporary depinning occurs for shear rate amplitudes above a frequency-dependent critical amplitude γ˙0crit(ω)\dot{\gamma}_0^\mathrm{crit}(\omega), for which we attain an approximate functional expression. For a range of frequencies, approaching γ˙0crit(ω)\dot{\gamma}_0^\mathrm{crit}(\omega) is accompanied by a strongly increasing settling time. Above γ˙0crit(ω)\dot{\gamma}_0^\mathrm{crit}(\omega), we further observe a variety of dynamical structures, whose stability exhibits an intriguing (γ˙0,ω\dot{\gamma}_0, \omega) dependence. This might enable new perspectives for potential control schemes.

Keywords

Cite

@article{arxiv.2207.05159,
  title  = {Depinning dynamics of confined colloidal dispersions under oscillatory shear},
  author = {Marcel Hülsberg and Sabine H. L. Klapp},
  journal= {arXiv preprint arXiv:2207.05159},
  year   = {2023}
}

Comments

17 pages, 11 figures