English

Decoupling environmental modes from tunneling electrons in a partially wet phase molecular mechanically controllable break junction

Mesoscale and Nanoscale Physics 2021-09-23 v3

Abstract

A quantum effect at ambient conditions is presented. A benzene dithiol (BDT) molecule or a tetrahydrofuran (THF) molecule is used as a barrier molecule bridging the gold electrodes from a Mechanically Controllable Break junction. It has been known for a long time that the environment of a junction couples to the conduction. With a microscopic layer of fluid it is actually possible to influence this coupling. The electrode-molecule-electrode configuration is lined with a microscopic layer of THF fluid, also known as the partially wet phase. This is effectively decoupling the electrode-molecule-electrode system from environmental modes outside of this system. The effects on coherence and quantum interference are exceptional.

Keywords

Cite

@article{arxiv.2106.01716,
  title  = {Decoupling environmental modes from tunneling electrons in a partially wet phase molecular mechanically controllable break junction},
  author = {C. J. Muller},
  journal= {arXiv preprint arXiv:2106.01716},
  year   = {2021}
}