English

Curvature Elasticity of the Electric Double Layer

Soft Condensed Matter 2018-08-06 v1

Abstract

Mean-field electrostatics is used to calculate the bending moduli of an electric double layer for fixed surface charge density of a macroion in a symmetric 1:1 electrolyte. The resulting expressions for bending stiffness, Gaussian modulus, and spontaneous curvature refer to a general underlying equation of state of the electrolyte, subject to a local density approximation and the absence of dipole and higher-order fields. We present results for selected applications: the lattice-gas Poisson-Fermi model with and without asymmetric ion sizes, and the Poisson-Carnahan-Starling model.

Keywords

Cite

@article{arxiv.1808.01180,
  title  = {Curvature Elasticity of the Electric Double Layer},
  author = {Guilherme Volpe Bossa and Bjorn K. Berntson and Sylvio May},
  journal= {arXiv preprint arXiv:1808.01180},
  year   = {2018}
}

Comments

5 pages, 4 figures. Published in Physical Review Letters. Copyright 2018 by the American Physical Society