English

Correlation and dimensional effects of trions in carbon nanotubes

Quantum Physics 2010-07-27 v1 Materials Science

Abstract

We study the binding energies of singlet trions, i.e. charged excitons, in carbon nanotubes. The problem is modeled, through the effective-mass model, as a three-particle complex on the surface of a cylinder, which we investigate using both one- and two-dimensional expansions of the wave function. The effects of dimensionality and correlation are studied in detail. We find that the Hartree-Fock approximation significantly underestimates the trion binding energy. Combined with band structures calculated using a non-orthogonal nearest neighbour tight binding model, the results from the cylinder model are used to compute physical binding energies for a wide selection of carbon nanotubes. In addition, the dependence on dielectric screening is examined. Our findings indicate that trions are detectable at room temperature in carbon nanotubes with radius below 8{\AA}.

Keywords

Cite

@article{arxiv.1005.4040,
  title  = {Correlation and dimensional effects of trions in carbon nanotubes},
  author = {Troels F. Rønnow and Thomas G. Pedersen and Horia D. Cornean},
  journal= {arXiv preprint arXiv:1005.4040},
  year   = {2010}
}