English

Correlated electronic structure with uncorrelated disorder

Strongly Correlated Electrons 2018-12-26 v2 Disordered Systems and Neural Networks

Abstract

We introduce a computational scheme for calculating the electronic structure of random alloys that includes electronic correlations within the framework of the combined density functional and dynamical mean-field theory. By making use of the particularly simple parameterization of the electron Green's function within the linearized muffin-tin orbitals method, we show that it is possible to greatly simplify the embedding of the self-energy. This in turn facilitates the implementation of the coherent potential approximation, which is used to model the substitutional disorder. The computational technique is tested on the Cu-Pd binary alloy system, and for disordered Mn-Ni interchange in the half-metallic NiMnSb.

Keywords

Cite

@article{arxiv.1807.09582,
  title  = {Correlated electronic structure with uncorrelated disorder},
  author = {A. Östlin and L. Vitos and L. Chioncel},
  journal= {arXiv preprint arXiv:1807.09582},
  year   = {2018}
}
R2 v1 2026-06-23T03:13:54.447Z