English

Colossal magnon-phonon coupling in multiferroic Eu$_{0.75}$Y$_{0.25}$MnO$_3$

Materials Science 2007-10-23 v4 Strongly Correlated Electrons

Abstract

We report the spectra of magnetically induced electric dipole absorption in Eu0.75_{0.75}Y0.25_{0.25}MnO3_3 from temperature dependent far infrared spectroscopy (10-250 cm1^{-1}). These spectra, which occur only in the eae||a polarization, consist of two relatively narrow electromagnon features that onset at TFE=30T_{FE}=30 K and a broad absorption band that persists to temperatures well above TN=47T_N=47 K. The observed excitations account for the step up of the static dielectric constant in the ferroelectric phase. The electromagnon at 80 cm1^{-1} is observed to be strongly coupled to the nearby lowest optical phonon which transfers more than 1/2 of its spectral weight to the magnon. We attribute the origin of the broad background absorption to the two magnon emission decay process of the phonon.

Keywords

Cite

@article{arxiv.0704.3632,
  title  = {Colossal magnon-phonon coupling in multiferroic Eu$_{0.75}$Y$_{0.25}$MnO$_3$},
  author = {R. Valdés Aguilar and A. B. Sushkov and C. L. Zhang and Y. J. Choi and S. -W. Cheong and H. D. Drew},
  journal= {arXiv preprint arXiv:0704.3632},
  year   = {2007}
}

Comments

4 pages, 3 figures