We use inelastic neutron scattering to study energy and wave vector dependence of spin fluctuations in SrCo2As2, derived from SrFe2−xCoxAs2 iron pnictide superconductors. Our data reveals the coexistence of antiferromagnetic (AF) and ferromagnetic (FM) spin fluctuations at wave vectors QAF=(1,0) and QFM=(0,0)/(2,0), respectively. By comparing neutron scattering results with those of dynamic mean field theory calculation and angle-resolved photoemission spectroscopy experiments, we conclude that both AF and FM spin fluctuations in SrCo2As2 are closely associated with a flat band of the eg orbitals near the Fermi level, different from the t2g orbitals in superconducting SrFe2−xCoxAs2. Therefore, Co-substitution in SrFe2−xCoxAs2 induces a t2g to eg orbital switching, and is responsible for FM spin fluctuations detrimental to the singlet pairing superconductivity.
@article{arxiv.1902.10621,
title = {Coexistence of ferromagnetic and stripe antiferromagnetic spin fluctuations in SrCo$_2$As$_2$},
author = {Yu Li and Zhiping Yin and Zhonghao Liu and Weiyi Wang and Zhuang Xu and Yu Song and Long Tian and Yaobo Huang and Dawei Shen and D. L. Abernathy and J. L. Niedziela and R. A. Ewings and T. G. Perring and Daniel Pajerowski and Masaaki Matsuda and Philippe Bourges and Enderle Mechthild and Yixi Su and Pengcheng Dai},
journal= {arXiv preprint arXiv:1902.10621},
year = {2019}
}
Comments
6 pages, 4 figures, supplemental material available upon request, to be published in PRL