English

CeRu$_4$Sn$_6$: heavy fermions emerging from a Kondo-insulating state

Strongly Correlated Electrons 2012-03-07 v1

Abstract

The combination of low-temperature specific-heat and nuclear-magnetic-resonance (NMR) measurements reveals important information of the ground-state properties of CeRu4_4Sn6_6, which has been proposed as a rare example of a tetragonal Kondo-insulator (KI). The NMR spin-latticerelaxation rate 1/T11/T_1 deviates from the Korringa law below 100 K signaling the onset of an energy gap ΔEg1/kB30\Delta E_g1/k_B \simeq 30K. This gap is stable against magnetic fields up to 10 T. Below 10 K, however, unusual low-energy excitations of in-gap states are observed, which depend strongly on the field H. The specific heat C detects these excitations in the form of an enhanced Sommerfeld coefficient γ=C(T)/T\gamma = C(T)/T : In zero field, γ\gamma increases steeply below 5 K, reaching a maximum at 0.1 K, and then saturates at γ=0.6\gamma = 0.6 J/molK2^2. This maximum is shifted to higher temperatures with increasing field suggesting a residual density of states at the Fermi level developing a spin gap ΔEg2\Delta E_g2. A simple model, based on two narrow quasiparticle bands located at the Fermi level - which cross the Fermi level in zero field at 0.022 states/meV f.u. - can account qualitatively as well as quantitatively for the measured observables. In particular, it is demonstrated that fitting our data of both specific heat and NMR to the model, incorporating a Ce magnetic moment of μ=ΔEg1/μ0H1μB\mu = \Delta E_g1/\mu_{0H} \simeq 1 \mu_B, leads to the prediction of the field dependence of the gap. Our measurements rule out the presence of a quantum critical point as the origin for the enhanced γ\gamma in CeRu4_4Sn6_6 and suggest that this arises rather from correlated, residual in-gap states at the Fermi level. This work provides a fundamental route for future investigations into the phenomenon of narrow-gap formation in the strongly correlated class of system

Keywords

Cite

@article{arxiv.1005.4912,
  title  = {CeRu$_4$Sn$_6$: heavy fermions emerging from a Kondo-insulating state},
  author = {E. M. Brüning and M. Brando and M. Baenitz and A. Bentien and A. M. Strydom and R. E. Walstedt and F. Steglich},
  journal= {arXiv preprint arXiv:1005.4912},
  year   = {2012}
}

Comments

11 pages, 13 figures