English

Cavity ringdown spectroscopy at 2 ${\mu}$m wavelength assisted by a comb-locked optical parametric oscillator

Optics 2025-05-30 v1 Atomic Physics

Abstract

We report on a comb-locked cavity ring-down spectrometer developed for high-precision molecular spectroscopy at 2 μ{\mu}m. It is based on the use of an external-cavity diode laser that is offset-frequency locked to the signal output of a singly-resonant optical parametric oscillator. This latter acts as reference laser, being locked to a self-referenced optical frequency comb, which in turn is stabilized against a GPS-disciplined Rb-clock. The performance of the spectrometer is investigated by probing a pair of N2_2O transitions belonging to hot vibrational bands. One of these, never observed before, is included in the N2_2O line list of the ExoMol database. Absolute center frequencies are retrieved with a 1-σ{\sigma} global uncertainty of 108 kHz.

Keywords

Cite

@article{arxiv.2505.23418,
  title  = {Cavity ringdown spectroscopy at 2 ${\mu}$m wavelength assisted by a comb-locked optical parametric oscillator},
  author = {Vittorio D'Agostino and Eugenio Fasci and Muhammad Asad Khan and Stefania Gravina and Livio Gianfrani and Antonio Castrillo},
  journal= {arXiv preprint arXiv:2505.23418},
  year   = {2025}
}