English

BaF molecules in neon ice: trapping, spectroscopy and optical control of electron spins

Atomic Physics 2023-08-02 v2

Abstract

We have trapped BaF molecules in neon ice, and used laser-induced fluorescence spectroscopy to map out optical transitions in the trapped molecules. Our measurements show that the neon lattice does not significantly perturb certain optical transitions in the trapped molecules. We used one of these transitions to polarize the electron spins, detect spin flips and measure hyperfine transitions in the trapped molecules, entirely using lasers. This demonstration with heavy polar molecules opens up new opportunities for precision measurements of beyond-standard-model physics.

Keywords

Cite

@article{arxiv.2207.07279,
  title  = {BaF molecules in neon ice: trapping, spectroscopy and optical control of electron spins},
  author = {Samuel J. Li and Harish D. Ramachandran and Rhys Anderson and Amar C. Vutha},
  journal= {arXiv preprint arXiv:2207.07279},
  year   = {2023}
}