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Atomic mass determination of uranium-238

Atomic Physics 2023-12-29 v1 Nuclear Experiment

Abstract

The atomic mass of uranium-238 has been determined to be 238.050787618(15)u238.050\,787\,618(15)\,\text{u}, improving the literature uncertainty by two orders of magnitude. It is obtained from a measurement of the mass ratio of 238^{238}U47+^{47+} and 132^{132}Xe26+^{26+} ions with an uncertainty of 3.5×10123.5\times 10^{-12}. The measurement was carried out with the Penning-trap mass spectrometer \textsc{Pentatrap} and was accompanied by a calculation of the binding energies EUE_{\text{U}} and EXeE_{\text{Xe}} of the 47 and 26 missing electrons of the two highly charged ions, respectively. These binding energies were determined using an \textit{ab initio} multiconfiguration Dirac-Hartree-Fock (MCDHF) method to be EU=39927(10)eVE_{\text{U}} = 39\,927(10)\,\text{eV} and EXe=8971.2(21)eVE_{\text{Xe}} = 8\,971.2(21)\,\text{eV}. The new mass value will serve as a reference for high-precision mass measurements in the heavy mass region of the nuclear chart up to transuranium nuclides.

Keywords

Cite

@article{arxiv.2312.17041,
  title  = {Atomic mass determination of uranium-238},
  author = {Kathrin Kromer and Chunhai Lyu and Jacek Bieroń and Menno Door and Lucia Enzmann and Pavel Filianin and Gediminas Gaigalas and Zoltán Harman and Jost Herkenhoff and Wenjia Huang and Christoph H. Keitel and Sergey Eliseev and Klaus Blaum},
  journal= {arXiv preprint arXiv:2312.17041},
  year   = {2023}
}

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Includes a Supplemental Material