English

Association between projectile and target excitation in slow Ar$^{q+}$-CO$_2$ collisions

Atomic Physics 2026-04-13 v1

Abstract

We investigate ionic fragmentation of CO2n+_2^{n+}~\mbox{(2n42\le n\le 4)} produced in collisions with Arq+^{q+}~\mbox{(4q164\le q\le 16)} projectiles at a collision velocity of \approx~0.3~a.u. For most projectile and fragmentation channel combinations, the shape of the kinetic energy release distribution (KERD) differs with the electron capture mediated charge change (\mbox{Δq\Delta q}) in the scattered projectile: KERD for \mbox{Δq=2\Delta q = 2} is broader at high KER than for \mbox{Δq=1\Delta q =1}. The difference generally diminishes with increasing projectile charge. Two deviations in this general trend are seen in the fragmentation of CO23+_2^{3+}, one for Ar4+^{4+} impact in the high KER region and the other for Ar6+^{6+} impact in the low KER region. The calculated reaction windows for multielectron capture within the framework of the extended classical over-the-barrier model (ECOBM) indicate that while ionization of the target occurs via multielectron capture, the scattered projectile may subsequently undergo multi-fold autoionization. Interpreting projectile autoionization to be a consequence of capture into highly excited states and high fragment KER to be a consequence of excitation of the ionized target to high-lying states, we find a strong dependence between the target and scattered projectile excitations.

Cite

@article{arxiv.2604.09348,
  title  = {Association between projectile and target excitation in slow Ar$^{q+}$-CO$_2$ collisions},
  author = {Akash Srivastav and Sumit Srivastav and Vishnu P and Bhas Bapat},
  journal= {arXiv preprint arXiv:2604.09348},
  year   = {2026}
}

Comments

Submitted to Phys. Rev. A